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Characterization of the performances of an innovative heat-exchanger/reactor

Theron, Félicie and Anxionnaz-Minvielle, Zoé and Cabassud, Michel and Gourdon, Christophe and Tochon, Patrice Characterization of the performances of an innovative heat-exchanger/reactor. (2014) Chemical Engineering and Processing: Process Intensification, 82. 30-41. ISSN 0255-2701

(Document in English)

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Official URL: http://dx.doi.org/10.1016/j.cep.2014.04.005


The use of heat exchanger/reactors (HEX/reactors) is a promising way to overcome the barrier of poor heat transfer in batch reactors. However to reach residence time long enough to complete the chemistry,low Reynolds number has to be combined with both a plug flow behaviour and the intensification of heat and mass transfers. This work concerns the experimental approach used to characterize an innovative HEX/reactor. The pilot is made of three process plates sandwiched between five utility plates. The process stream flows in a 2 mm corrugated channel. Pressure drop and residence time distribution characterizations aim at studying the flow hydrodynamics. Identified Darcy correlations point out the transition between laminar and turbulent flow around a Reynolds number equal to 200. Moreover the flow behaves like a quasi-plug flow (Pe > 185). The heat transfer and mixing time have also been investigated. The ratio between the reaction kinetics and the mixing time is over 100 and the intensification factor ranges from5000 to 8000 kW m−3K−1. As a consequence, no limitations were identified which allows the implementation of an exothermic reaction. It has been successfully performed under severe temperature and concentration conditions, batchwise unreachable. Thus, it highlights the interest of using this continuous HEX/reactor.

Item Type:Article
Additional Information:Thanks to Elsevier editor. The definitive version is available at http://www.sciencedirect.com The original PDF of the article can be found at Chemical Engineering and Processing website : http://www.sciencedirect.com/science/journal/02552701
HAL Id:hal-01346088
Audience (journal):International peer-reviewed journal
Uncontrolled Keywords:
Institution:French research institutions > Commissariat à l'Energie Atomique et aux énergies alternatives - CEA (FRANCE)
French research institutions > Centre National de la Recherche Scientifique - CNRS (FRANCE)
Université de Toulouse > Institut National Polytechnique de Toulouse - Toulouse INP (FRANCE)
Université de Toulouse > Université Toulouse III - Paul Sabatier - UT3 (FRANCE)
Laboratory name:
Deposited On:18 Jul 2016 10:30

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